[P-087]
RELATIONSHIP BETWEEN LIPOPHILICITY OF NATURALLY OCCURING FLAVONOLS AND THE RETENTION IN REVERSED PHASE LIQUID CHROMATOGRAPHY

B. Dimitrova1, Reneta Gevrenova2 and I. Doytchinova1
1Faculty of Pharmacy, Department of Chemistry, 2, Dunav Str., 1000 Sofia, Bulgaria
2Faculty of Pharmacy, Department of Pharmacognosy and Botany, 2 Dunav Str., 1000 Sofia, Bulgaria

The flavonol glycosides from Bupleurum flavum Forsk., Apiaceae, are separated isocratically and identified by LC-MS. The obtained results revealed the presence of quercetin-dirhamnoside, quercetin-3-rhamnosylglucoside, quercetin-3-glucoside, iso-rhamnetin-3-rhamnosylglucoside, kaempferol-dirhamnoside, kaempferol-3-glucoside. The RP-HPLC behaviour of the flavonol glycosides is tested on Supersphere RP18, 4 mm and Hypersil ODS, 5 mm packing materials sequentially varying the composition of the aqueous/methanol mobile phase. To improve of the separation the effect of small amount of butanol isomers - iso-BuOH, sec-BuOH, n-BuOH and t-BuOH - in the eluent is examined also and the influence of the buffer system. Further, the relationship between the capacity factors log k' obtained in the RP-HPLC system for the plant extracted glycosides and the lipophilicity parameters CLOGP calculated for n-octanol-water system by the computer program ACD/logP is studied. Good correlations are established. The results indicate that the increasing of the content of tret-BuOH leads to higher values of the regression coefficient R and the same is valid for the buffer concentration. One may conclude that the RP-HPLC system with higher contents of t-BuOH and buffer imitates well the partition behavior of the glycosides in the n-octanol-water system. In the present study the best result is found for the composition of 70% buffer and 7% t-BuOH.

[Full paper: P-087]
[P-087]